4.6 Article

Controlled directional ion emission from several fragmentation channels of CO driven by a few-cycle laser field

期刊

PHYSICAL REVIEW A
卷 86, 期 6, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.86.063403

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资金

  1. Max Planck Society
  2. Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, US Department of Energy [DE-FG02-86ER13491, DE-FG02-00ER15053]
  3. National Science Foundation [CHE-0822646]
  4. DFG
  5. International Collaboration in Chemistry program
  6. Cluster of Excellence: Munich Center for Advanced Photonics (MAP)
  7. EU via LaserLab Europe
  8. Fulbright Commission
  9. Division Of Chemistry
  10. Direct For Mathematical & Physical Scien [0822646] Funding Source: National Science Foundation
  11. U.S. Department of Energy (DOE) [DE-FG02-00ER15053] Funding Source: U.S. Department of Energy (DOE)

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We explore the dissociative ionization of CO with carrier-envelope-phase (CEP) tagged few-cycle laser pulses. We observe the CEP dependence of the directional emission of Cp+ and Oq+ fragments from transient CO(p+q)+ ions, where p + q <= 3 and q <= 1. At I-0 = 3.5 x 10(14) W/cm(2), a 180 degrees phase difference between the C+ and O+ fragments from the (p = 1, q = 0) and (p = 0, q = 1) channels reflects the orientation dependence of the CO ionization. At I-0 = 1.2 x 10(15) W/cm(2), we find a similar to 35 degrees phase shift between the C2+ fragments from the (p = 2, q = 0) and (p = 2, q = 1) channels, in contrast to the 180 degrees shift previously observed between the C2+ fragment channels at I-0 = 6 x 10(14) W/cm(2) [Phys. Rev. Lett. 106, 073004 (2011)]. DOI: 10.1103/PhysRevA.86.063403

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