期刊
PHYSICAL REVIEW A
卷 82, 期 2, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.82.023413
关键词
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资金
- US Department of Energy [DE-FG02-04ER15612]
- Keck Foundation [705343]
- U.S. Department of Energy (DOE) [DE-FG02-04ER15612] Funding Source: U.S. Department of Energy (DOE)
We introduce an optimal control approach that is capable of yielding the best achievable field-free three-dimensional (3-D) alignment in an arbitrary molecule. Our analysis provides the optimal route to the best aligned state along with interesting insights into the 3-D alignment dynamics of polyatomic systems.
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