期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 16, 期 26, 页码 13063-13068出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cp01503g
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资金
- Engineering and Physical Sciences Research Council (U.K.) EPSRC(GB)
- [EP/J003085/1]
- EPSRC [EP/J003085/1, EP/I00422X/1, EP/J016454/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/J003085/1, EP/J016454/1, EP/I00422X/1] Funding Source: researchfish
In situ and ex situ Raman analyses of porous Ni/CGO electrodes reveal differences in the amount, location and type of carbon formed during CO/CO2 electrolysis. The results demonstrate the limitations of optical in situ techniques applied to Solid Oxide Cells (SOCs) operated in electrolysis conditions. Increased carbon deposition close to the electrode-electrolyte interface is likely to be the result of high chargetransfer current in that area. The positive effect of a CGO interlayer on reducing carbon formation on the fuel electrode is demonstrated.
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