期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 16, 期 28, 页码 14640-14643出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cp01531b
关键词
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资金
- U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DESC0006647]
- Materials Research Science and Engineering Center program of the National Science Foundation [DMR 1120296]
Sub-10 nm monodisperse PbS cubes are synthesized by reacting quasi-spherical PbS nanocrystals with (NH4)(2)S. This reaction shapes the quasi-spheres into cubes via preferential growth of the (111) facets. A four-band envelope function calculation of the energy levels accounts well for the measured absorption spectra. Initial studies show that PbS cubes can organize into simple square superlattices with short ligands.
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