期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 15, 期 29, 页码 12165-12172出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cp50707f
关键词
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资金
- MICINN [RYC-2009-04199]
- Consejeria de Ciencia e Innovacion, Junta de Andalucia [CTQ2011-28954-C02-02, P10-FQM-6711]
Cu nanoparticles have been supported by two types of aluminosilicate materials with and without Zn in their composition in view of their application in the microwave-assisted conversion of glucose to valuable products via tandem formic acid-promoted dehydration (to 5-hydroxymethylfurfural-HMF) and further selective hydrogenation to 5-methylfurfuryl alcohol (MFA). Results show that interesting selectivities (up to 60% to MFA or HMF) could be achieved after short times of reaction (typically 2-30 min) using Cu-containing nanomaterials. Zn was found to play an interesting role in the selectivity to reduced products, even if present in very small quantities (0.2 wt%).
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