期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 15, 期 26, 页码 10580-10611出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cp50620g
关键词
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资金
- Center for Nanophase Materials Sciences
- Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy
- World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan
- Core Research for Evolutional Science and Technology (CREST) program of Japan Science and Technology Agency (JST), Japan
Amphiphiles, either synthetic or natural, are structurally simple molecules with the unprecedented capacity to self-assemble into complex, hierarchical geometries in nanospace. Effective self-assembly processes of amphiphiles are often used to mimic biological systems, such as assembly of lipids and proteins, which has paved a way for bottom-up nanotechnology with bio-like advanced functions. Recent developments in nanostructure formation combine simple processes of assembly with the more advanced concept of nanoarchitectonics. In this perspective, we summarize research on self-assembly of amphiphilic molecules such as lipids, surfactants or block copolymers that are a focus of interest for many colloid, polymer, and materials scientists and which have become increasingly important in emerging nanotechnology and practical applications, latter of which are often accomplished by amphiphile-like polymers. Because the fundamental science of amphiphiles was initially developed for their solution assembly then transferred to assemblies on surfaces as a development of nanotechnological techniques, this perspective attempts to mirror this development by introducing solution systems and progressing to interfacial systems, which are roughly categorized as (i) basic properties of amphiphiles, (ii) self-assembly of amphiphiles in bulk phases, (iii) assembly on static surfaces, (iv) assembly at dynamic interfaces, and (v) advanced topics from simulation to application. This progression also represents the evolution of amphiphile science and technology from simple assemblies to advanced assemblies to nanoarchitectonics.
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