期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 14, 期 28, 页码 9988-9995出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cp40695k
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资金
- ANCyPT [PICT 1146, PAE 2004, 22711, PAE-2006, 37063]
- CONICET
Experimental evidence of the variation in redox potential of osmium pyridine complexes tethered to a Au surface by thiol or diazonium chemistry at different ionic concentration and electrolyte pH is described. The interplay between the charged redox and acid groups is described by a charge regulation model based on PM-IRRAS spectroscopic evidence on the different degrees of surface protonation.
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