期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 13, 期 43, 页码 19307-19309出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cp22817j
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资金
- Robert Bosch (SEA) Pte Ltd
- National Research Foundation, Singapore
A solution processed method for fabricating transition metal sulfides on fluorine doped tin oxide (FTO) as efficient counter electrodes in iodine/iodide based solar cells has been demonstrated. Conversion efficiencies of 7.01% and 6.50% were obtained for nickel and cobalt sulfides, respectively, comparable to the conventional thermally platinised FTO electrodes (7.32%). A comparable charge transfer resistance of Ni3S2 and Co8.4S8 to conventional Pt was found to be a key factor for such high efficiencies. Cyclic voltammetry, Kelvin probe microscopy, Electrochemical Impedance Spectroscopy, and Tafel polarization were performed to study the underlying reasons behind such efficient counter electrode performance.
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