期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 10, 期 24, 页码 3561-3568出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b801838c
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We report on thermodynamic modeling and computer simulations on the electrochemical generation of metallic and bimetallic nanoparticles (NPs) by means of quenched molecular dynamics (QMD). The present results suggest that the spontaneous formation of core-shell NPs depends on several factors, i.e. size and shape of the core, chemical composition of the system, and under-/oversaturation conditions. Homo- and heteroatomic prototypical systems were considered. The former systems were Au and Pt. The latter were Ag(core)/Au(shell), Pt(core)/Au( shell), Au( core)/Ag(shell) and Au(core)/Pt(shell).
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