期刊
PHOTOSYNTHESIS RESEARCH
卷 102, 期 2-3, 页码 255-266出版社
SPRINGER
DOI: 10.1007/s11120-009-9483-6
关键词
X-ray spectroscopy; X-ray emission; Synchrotron radiation; Electronic structure; Photosystem II; Manganese; Oxygen evolving complex
We describe the chemical information that can be obtained by means of hard X-ray emission spectroscopy (XES). XES is presented as a technique that is complementary to X-ray absorption spectroscopy (XAS) and that provides valuable information with respect to the electronic structure (local charge- and spin-density) as well as the ligand environment of a 3d transition metal. We address non-resonant and resonant XES and present results that were recorded on Mn model systems and the Mn4Ca-cluster in the oxygen evolving complex of photosystem II. A brief description of the instrumentation is given with an outlook toward future developments.
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