期刊
ORGANOMETALLICS
卷 30, 期 21, 页码 5556-5559出版社
AMER CHEMICAL SOC
DOI: 10.1021/om2008138
关键词
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资金
- EPSRC (U.K.)
- EPSRC [EP/I014519/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/I014519/1] Funding Source: researchfish
Reaction of catalytic quantities of a beta-diketiminato n-butylmagnesium complex with pinacol-borane in the presence of pyridine derivatives provides facile access to borylated dihydropyridines. The reaction is applicable to a wide range of monocyclic and fused-ring pyridine derivatives and catalytic turnover is proposed to occur through a well-defined sequence of Mg-H/pyridine dearomatization and Mg-N/B-H sigma bond metathesis steps.
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