期刊
ORGANOMETALLICS
卷 28, 期 13, 页码 3856-3862出版社
AMER CHEMICAL SOC
DOI: 10.1021/om900120v
关键词
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资金
- National Natural Science Foundation of China [20632040]
- Department of National Education Doctoral Foundation
A series of new trisguanidinate lanthanide complexes including the first THF-solvated trisguanidinate lanthanum complexes were synthesized and fully characterized. The complexes were found to be efficient catalysts for amidation of aldehydes with amines under mild conditions with a wide scope of substrates including pyrrolidine, piperidine, and morpholine, and one of the intermediates for this process, lanthanum amido complex {[((PrN)-Pr-i)(CNHPr)-Pr-i(NC(6)H(4)p-Cl)](2)La(NHC6H5)}(2)center dot C7H8, was isolated.
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