期刊
ORGANIC LETTERS
卷 16, 期 6, 页码 1732-1735出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol5004093
关键词
-
资金
- National Natural Science Foundation of China [21032001, 21272085]
- Central China Normal University [2013YBYB58]
A highly efficient and selective molecular iodine-promoted oxidative cross-coupling/annulation between 2-naphthols and methyl ketones has been realized. The reaction successfully constructed a new quaternary carbon center within 3(2H)-furanones. Our synthetic strategy provided an in situ iodination-based oxidative coupling pathway. Based on the experimental results, a self-sequenced iodination/Kornblum oxidation/Friedel-Crafts/oxidation/cyclization mechanism was proposed.
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