期刊
ORGANIC LETTERS
卷 16, 期 3, 页码 1004-1007出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol403746r
关键词
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资金
- JSPS [22249001, 25460017, 21790019]
- MEXT [2105, 22106538, 24106736]
- Naito Foundation
- Grants-in-Aid for Scientific Research [25253002, 25460017, 22106538, 24105526, 24659009, 21790019, 24106736] Funding Source: KAKEN
A novel formal [4 + 1]-cycloaddition of readily available homopropargyl alcohols with diazo dicarbonyl compounds is described, which involves tandem O-H insertion/Conia-ene cyclization under cooperative Rh(II)/Zn(II) catalysis. This reaction provides easy access to various substituted tetrahydrofurans and exhibits complete E-selectivity in the case of nonterminal alkynes.
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