期刊
ORGANIC LETTERS
卷 15, 期 11, 页码 2730-2733出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol401065r
关键词
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资金
- Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio)
- Energy Frontier Research Center
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC0000997]
Phenolic lignin model monomers and dimers representing the primary substructural units of lignin were successfully oxidized to benzoquinones in high yield with molecular oxygen using new Co-Schiff base catalysts bearing a bulky heterocyclic nitrogen base as a substituent. This is the first example of a catalytic system able to convert both S and G lignin model phenols in high yield, a process necessary for effective use of lignin as a chemical feedstock.
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