期刊
ORGANIC LETTERS
卷 15, 期 22, 页码 5698-5701出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol4027107
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资金
- Pfizer Worldwide Research and Development
- BP 1702 endowment
A flow chemistry process for the Oppenauer oxidation of benzylic secondary alcohols using partially hydrated zirconium oxide and a simple carbonyl containing oxidant such as acetone, cyclohexanone, and neopentanal is reported. The heterogeneous oxidative system could be applied to a wide range of functionalized alcohol substrates, allowing clean and fast delivery of ketone products within a few minutes between 40 and 100 degrees C.
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