期刊
ORGANIC LETTERS
卷 15, 期 22, 页码 5822-5825出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol402877n
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资金
- Singapore National Research Foundation (NRF)
- Economic Development Board (EDB)
- GlaxoSmithKline (GSK)
- Nanyang Technological University (NTU)
An NHC-catalyzed activation of acetic esters to afford enolate intermediates is disclosed. The catalytically generated triazolium enolate intermediates serve as two-carbon nucleophiles that undergo highly enantioselective reactions with enones and alpha,beta-unsaturated imines to give a-unsubstituted delta-lactones and lactams, respectively.
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