期刊
ORGANIC LETTERS
卷 15, 期 17, 页码 4600-4603出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol4022113
关键词
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资金
- National Basic Research Program of China [2011CB808600]
- National Natural Science Foundation of China [21102073, 21072093, 20932004]
Copper-catalyzed cross-dehydrogenative coupling (CDC) reactions of (benzo)thiazoles with cyclic ethers were developed under mild conditions. In particular, the formation of C-C bonds via the CDC reactions between non-benzo-fused azoles and ethers are reported for the first time. In addition, the acetals, known as the masked 2-thiazolecarboxaldehydes, could be successfully obtained by this CDC reaction. The preliminary mechanism and supportive DFT calculations are discussed as well.
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