期刊
ORGANIC LETTERS
卷 15, 期 6, 页码 1250-1253出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol400184t
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资金
- EU [PIIF-GA-2010-274903]
- Skaggs-Oxford Scholarship Program
- NSF GRFP
- EPSRC
- GSK
- CONACyT Mexico Program [205456]
- BBSRC
- Biotechnology and Biological Sciences Research Council [1112421] Funding Source: researchfish
- Engineering and Physical Sciences Research Council [1250529] Funding Source: researchfish
A new catalytic method to access allylic secondary CF3 products is described. These reactions use the visible light excited Ru(bpy)(3)Cl-2 center dot 6H(2)O catalyst and the Togni or Umemoto reagent as the CF3 source. The photoredox catalytic manifold delivers enantioenriched allylic trifluoromethylated products not accessible under Cu(I) catalysis.
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