期刊
ORGANIC LETTERS
卷 15, 期 23, 页码 6002-6005出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol402890m
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资金
- NSERC
- ACS PRF
- Bayer CropScience
- Canada Research Chairs program
Chemoselectivity of intramolecular hydroaminoalkylation over hydroamination has been achieved with a bis(3-phenyl-2-pyridonate) titanium complex. Primary aminoalkenes are selectively alpha-alkylated by C-H functionalization adjacent to nitrogen to access five- and six-membered cycloalkylamines with a good substrate-dependent diastereoselectivity of up to 19:1.
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