期刊
ORGANIC LETTERS
卷 15, 期 5, 页码 1028-1031出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol303512f
关键词
-
资金
- [ANR-08-blan-0186-01]
Dissymmetric pi-conjugated monomers and oligomers incorporating 3,4-ethylenedioxythiophene (EDOT) units and bearing terpyridine end groups were synthesized in good yields through Vilsmeyer-Haak formylation followed by a reaction with 2-acetylpyridine in basic media or, for the longest oligomers, direct C H bond arylation. They have a low HOMO-UMO gap and are easily oxidized at low potentials. Upon complexation with cobalt(II) and iron(II) they yield new hybrid materials that can be used in various applications ranging from photovoltaics to spintronics.
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