期刊
ORGANIC LETTERS
卷 15, 期 3, 页码 476-479出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol303263q
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资金
- UCSB
- National Science Foundation (CAREER Award) [CHE-1057180]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1057180, 1040541] Funding Source: National Science Foundation
The first example of a Piancatelli rearrangement of alcohols is demonstrated utilizing dysprosium(III) trif late as a catalyst to access oxaspirocycles in a highly diastereoselective manner. The cascade reaction constructs the spirocyclic ether ring system and the tertiary stereocenter in a single operation and is experimentally easy to perform.
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