期刊
ORGANIC LETTERS
卷 14, 期 8, 页码 2164-2167出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol3006997
关键词
-
资金
- NSFC [20872126, 21072169]
- Fundamental Research Funds for the Central Universities [2010QNA3011]
Thioethers have been proven to be reliable directing groups for palladium catalyzed alkenylation of arenes via C-H activation. Mechanistic investigation reveals that the C-H cleavage of arenes is the turnover-limiting step, and an acetate-bridged dinuclear cyclopalladation intermediate is involved. The alkenylated thioethers can be easily removed and transformed into a variety of useful groups.
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