期刊
ORGANIC LETTERS
卷 14, 期 16, 页码 4054-4057出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol301559k
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资金
- Western Light Talent Culture Project
- Sichuan Youth Science and Technology Foundation
An efficient FeCl3-catalyzed stereoselective intramolecular tandem 1,5-hydride transfer/ring closure reaction was developed. The method allows for the formation of structurally diverse spirooxindole tetrahydroquinolines in high yields (up to 98%) with good to excellent levels of diastereoselectivity (up to 99:1 dr). The catalytic enantioselective variant of this process was also investigated preliminarily with a chiral BINOL-derived phosphoric acid.
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