期刊
ORGANIC LETTERS
卷 14, 期 11, 页码 2838-2841出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol301077y
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资金
- Department of Science and Technology (DST), New Delhi, India
- Department of Atomic Energy (DAE-BRNS) Mumbai
- IISER Bhopal
Synthesis of substituted phenanthridinones and dibenzoazepinones has been realized from 2-halo-benzamides in the presence of potassium tert-butoxide and a catalytic amount of 1,10-phenanthroline or AIBN. This new carbon-carbon bond forming reaction gives direct access to various blaryl lactams containing six- and seven-membered rings chemoselectively. Carbon-carbon coupling seems to proceed by the generation of a radical In the amide ring which leads to C-H arylation of aniline.
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