期刊
ORGANIC LETTERS
卷 14, 期 7, 页码 1720-1723出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol3002877
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-
资金
- National Institutes of Health [GM062924]
Vinyl sulfides react rapidly and efficiently with 2,3-dichloro-5,6-dicyano-1,4-benzoquinone (DDQ) to form alpha,beta-unsaturated thiocarbenium ions through oxidative carbon-hydrogen bond cleavage. These electrophiles couple with appended pi-nucleophiles to yield sulfur-containing heterocycles through carbon-carbon bond formation. Several nucleophiles are compatible with the procedure, and the reactions generally proceed through readily predictable transition states.
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