期刊
ORGANIC LETTERS
卷 14, 期 21, 页码 5546-5549出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol302640e
关键词
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资金
- National Natural Science Foundation of China [21072047, 21172059, 21272059, 21202039]
- Program for New Century Excellent Talents in University of Ministry of Education [NCET-09-0122]
- Excellent Youth Foundation of Henan Scientific Committee [114100510012]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT1061]
- Program for Innovative Research Team in University of Henan Province [2012IRTSTHN006]
- Henan Normal University
A new method for C-C and C-N bond formation of heteroaromatics and C(sp(3))-H alkanes was developed with high regioselectivity. The reaction occurred on C8 to give 8-cylcoakylpurines by C-C bond formation only promoted by tBuOOtBu, while it occurred on the amino group to give N6-alkylated purines by C-N bond formation when 2 equiv of Cul were added. A reaction mechanism was also proposed based on our preliminary experimental data.
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