期刊
ORGANIC LETTERS
卷 14, 期 9, 页码 2406-2409出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol300832f
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资金
- Deutsche Forschungsgemeinschaft [Oe 249/3-2]
- Fonds der Chemischen Industrie
The two-directional desymmetrization of prochiral precursors with alpha,beta-unsaturated branches by catalyst-controlled 1,4-addition of silicon and likewise boron nucleophiles allows for a general enantioselective access to syn,anti-triols with 1,n + 1,2n + 1 (n = 2 and 3) substitution patterns. The utility is demonstrated in the synthesis of the C17-C25 fragment of dermostatin A.
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