期刊
ORGANIC LETTERS
卷 15, 期 2, 页码 258-261出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol303073b
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资金
- EPSRC [EP/G068313/1]
- University of York Wild Fund
- University Strategic Equipment Fund
- Engineering and Physical Sciences Research Council [EP/G068313/1, EP/J016128/1] Funding Source: researchfish
- EPSRC [EP/G068313/1, EP/J016128/1] Funding Source: UKRI
A simple and efficient procedure to prepare a range of diverse heterocycles by the direct acylation of imines using a variety of functionalized benzoic acids is described. The methodology features a novel method for N-acyliminium ion generation followed by in situ intramolecular trapping by oxygen-, nitrogen-, sulfur- and carbon-based nucleophiles. Preliminary mechanistic studies, using ReactIR, are also reported.
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