期刊
ORGANIC LETTERS
卷 14, 期 4, 页码 988-991出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol203224n
关键词
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资金
- Fundacao para a Ciencia e Tecnologia [PTDC/QUI-QUI/118315/2010, PTDC/QUI-QUI/099389/2008, FRH/BPD/46589/2008, FRH/BPD/48219/2008, Pest-OE/SAU/UI4013/2011, PEst-OE/QUI/UI0100/2011]
- Fundação para a Ciência e a Tecnologia [PTDC/QUI-QUI/099389/2008, PTDC/QUI-QUI/118315/2010] Funding Source: FCT
The dative N-B bond was used to simply assemble heterocycles with a skeleton akin to the 5-oxofuro[2,3-b]furan motif. Twenty-five new N-B heterocycles were prepared via a highly efficient one-pot four-component reaction in yields and diastereoselectivities up to 95% and >97%, respectively. Several reaction intermediates were discovered using electrospray ionization mass spectroscopy which set the basis for the mechanism elucidation using DFT calculations.
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