期刊
ORGANIC LETTERS
卷 14, 期 21, 页码 5492-5495出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol302570k
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资金
- Clare College, Cambridge
The total synthesis of the cAMP signaling pathway activator (-)-alotaketal A is reported. A convergent approach to the unusual alotane sesterterpenoid skeleton was employed, exploiting a remarkable LiDBB-mediated coupling of an (R)-carvone-derived delta-lactone with an allyl bromide side chain, followed by spiroacetalization.
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