期刊
ORGANIC LETTERS
卷 14, 期 4, 页码 1110-1113出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol3000298
关键词
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资金
- NIH [GM095666, RR08389-01]
- Sloan Foundation
- NSF [CHE-9208463, CHE-9629688]
alpha,beta-Unsaturated 2-imidazolyl ketones undergo [2 + 2] cycloaddition with a variety of Michael acceptors upon irradiation with visible light in the presence of Ru(bpy)(3)(2+). Cleavage of the imidazolyl auxiliary from the cycloadducts affords cyclobutane carboxamides, esters, thioesters, and acids that would not be accessible from direct cycloaddition of the corresponding unsaturated carbonyl compounds.
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