期刊
ORGANIC LETTERS
卷 14, 期 17, 页码 4556-4559出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol302023q
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资金
- National Science Foundation [CHE-0955864]
- Boehringer Ingelheim
- DuPont
- Eli Lilly
- Amgen
- AstraZeneca
- Roche
- Sloan Foundation
- University of California, Los Angeles
- NSF [CHE-1048804]
- National Center for Research Resources [S10RR025631]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0955864] Funding Source: National Science Foundation
A concise approach toward the total synthesis of the communesin alkaloids and perophoramidine is reported. The strategy relies on the use of the interrupted Fischer indolization to build the tetracyclic indoline core of the natural products. Studies to probe the scope and limitations of this plan are presented. Although the methodology does not tolerate a C8-allyl substituent en route to the challenging vicinal quaternary stereocenters, variation at Cl and on the C ring is permitted.
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