期刊
ORGANIC LETTERS
卷 14, 期 6, 页码 1428-1431出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol300173v
关键词
-
资金
- National Institute of Health [CA042056, CA115526, CA165303]
An Fe(III)/NaBH4-mediated reaction for the functionalization of unactivated alkenes is described defining the alkene substrate scope, establishing the exclusive Markovnikov addition, exploring a range of free radical traps, examining the Fe(III) salt and initiating hydride source, introducing H2O-cosolvent mixtures, and exploring catalytic variants. Its use led to the preparation of a novel, potent, and previously inaccessible C20'-vinblastine analogue.
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