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ORGANIC LETTERS
卷 14, 期 14, 页码 3796-3799出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol301681z
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资金
- Boehringer Ingelheim
- DuPont
- Eli Lilly
- Amgen
- AstraZeneca
- Roche
- A. P. Sloan Foundation
- University of California, Los Angeles
- Foote Family fellowships
- CBI training program [GM08496]
- NSF [CHE-1048804]
- National Center for Research Resources [S10RR025631]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1048804] Funding Source: National Science Foundation
The alkylation of aryl sulfamates and carbamates using iron catalysis is reported. The method constructs sp(2)-sp(3) carbon-carbon bonds and provides synthetically useful yields across a range of substrates (>35 examples). The directing group ability of sulfamates and carbamates, accompanied by their low reactivity toward conventional cross-couplings, renders these substrates useful for the synthesis of polyfunctionalized arenes.
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