期刊
ORGANIC LETTERS
卷 14, 期 16, 页码 4110-4113出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol301759v
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资金
- AstraZeneca
- Chinese Scholarship Council
Cationic ruthenium(II) complexes enabled catalytic twofold C-H bond functionalizations with weakly coordinating aromatic esters in a highly chemo-, site- and diastereo-selective as well as site selective fashion. The oxidative Fujiwara-Moritani-type alkenylation provided step-economical access to diversely substituted styrenes and proved viable in an aerobic manner. Mechanistic studies were indicative of a reversible acetate-assisted cycloruthenation step.
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