期刊
ORGANIC LETTERS
卷 14, 期 1, 页码 98-101出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol2028866
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资金
- Specialized Research Fund for the Doctoral Program of Higher Education [20103201120006]
- NSFC [21102097]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
- Soochow University
- Jiangsu Province Higher Education Graduate Student Research and Innovation Project [CXLX11_0067]
An aerobic visible-light driven photoredox catalytic formation of 2-substituted benzothiazoles through radical cyclization of thioanilides has been accomplished. The reaction features C-H functionalization and C-S bond formation with no direct metal involvement except the sensitizer. The reaction highlights the following: (1) visible-light is the reaction driving force; (2) molecular oxygen is the terminal oxidant, and (3) water Is the only byproduct.
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