期刊
ORGANIC LETTERS
卷 13, 期 23, 页码 6204-6207出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol202629d
关键词
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资金
- Natural Science and Engineering Research Council (NSERC) of Canada
- Canadian Fund for Innovation (CFI)
- Universite de Sherbrooke
- FQRNT
- NSERC
- CGCC
The core of daphnilactone B-type and yuzurimine-type alkaloids was synthesized In only 16 steps from a known beta-allyl-gamma-butyrolactone. The key sequence of Vilsmeier-Haack cyclization and intramolecular azomethine ylide cycloaddition allowed the construction of, in a single step, three of the five rings common to all alkaloids found in both of these classes with perfect chemocontrol.
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