期刊
ORGANIC LETTERS
卷 13, 期 13, 页码 3506-3509出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol201314m
关键词
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资金
- JSPS [22350041]
- Grants-in-Aid for Scientific Research [22350041] Funding Source: KAKEN
An enantioselective intramolecular oxidative cyclization of 4-alkenoic acids was developed. The reaction proceeded via a pi-allyl Pd intermediate generated by an allylic C-H activation to give gamma-lactone derivatives with moderate to good enantioselectivity. Spiro bis(isoxazoline) ligand, SPRIX, was indispensable for this asymmetric transformation.
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