期刊
ORGANIC LETTERS
卷 14, 期 1, 页码 186-189出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol202971m
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资金
- University of California, Davis
- National Science Foundation [CHE-0847358]
- 3M Nontenured faculty
- United States Department of Education
- UC Davis
The importance of cooperative hydrogen-bonding effects and SIOH-acidification Is described for silanediol catalysis. NMR binding, X-ray, and computational studies provide support for a unique dimer resulting from silanediol self-recognition. The significance of this cooperative hydrogen-bonding Is demonstrated using novel fluorinated silanediol catalysts for the addition of indoles and N,N-dimethyl-m-anisidine to trans-beta-nitrostyrene.
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