期刊
ORGANIC LETTERS
卷 13, 期 7, 页码 1820-1823出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol200333p
关键词
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资金
- Ministry of Education, Culture, Sports, Science and Technology, Japan
- Grants-in-Aid for Scientific Research [23681045, 21241050, 23102016] Funding Source: KAKEN
Intramolecular oxa-conjugate cyclization of alpha,beta-unsaturated thioesters under Bronsted acid catalysis, inspired by biosynthesis of polyketide natural products, provides a variety of 2,6-cis-substituted tetrahydropyran derivatives with excellent diastereoselectivities. An added bonus of this methodology is that the product tetrahydropyrans could be readily elaborated to various derivatives by exploiting the unique reactivity of the thioester group.
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