期刊
ORGANIC LETTERS
卷 13, 期 5, 页码 1068-1071出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol103112v
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资金
- NIH [RO1-NIGMS]
- Amgen
- AstraZeneca
- GlaxoSmithKline
- GAANN
- FQRNT (Fonds Quebecois de la Recherche sur la Nature et les Technologies)
- U.S. Department of Energy [DE-AC02-06CH11357]
- Michigan Economic Development Corp. [085P1000817]
An NHC-catalyzed, diastereo- and enantioselective dimerization of enals has been developed. The use of Ti(Oi-Pr)(4) is a key element for the reactivity and selectivity of this process. The cyclopentenes are obtained with high levels of diastereo- and enantioselectivity and their synthetic utility is demonstrated by functionalization of the product alkene.
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