期刊
ORGANIC LETTERS
卷 12, 期 9, 页码 2124-2127出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol100619p
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资金
- EPSRC
- DSTL
Synthesis of fused bis-anthracene porphyrin monomers and dimers has been achieved by oxidative ring closure using FeCl3 and Sc(OTf)(3)/DDQ, respectively. The fused compounds display red-shifted absorption spectra with maxima in the near-IR at 973 and 1495 nm, respectively, and small electrochemical HOMO-LUMO gaps. The crystal structure of the fully fused bis-anthracene porphyrin shows that it has a regular planar pi-system.
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