期刊
ORGANIC LETTERS
卷 12, 期 13, 页码 3058-3061出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol1010888
关键词
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资金
- Ministerio de Ciencia e Innovacion
- FEDER [CTQ2006-14199, CTQ2009-13083]
- Generalitat Valenciana [ACOMP/2009/338]
- Universitat de Valencia
A catalytic highly enantioselective Henry addition of methyl 4-nitrobutyrate to aldehydes using a Cu(II) amino pyridine complex as catalyst is described. The products resulting from this reaction constitute a new, highly versatile family of chiral building blocks as a result of the presence of three different functional groups on the molecule. These products have been transformed into nonracemic chiral gamma-lactams, 5-hydroxy-5-substituted levulinic acid derivatives, and delta-lactones.
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