期刊
ORGANIC LETTERS
卷 12, 期 16, 页码 3682-3685出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol101490n
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资金
- Nanyang Technological University
- Singapore Ministry of Education
A copper-catalyzed synthesis of phenanthridine derivatives was developed starting from biaryl-2-carbonitriles and Grignard reagents. The present transformation is carried out by a sequence of nucleophilic addition of Grignard reagents to biaryl-2-carbonitriles to form N-H imines and their Cu-catalyzed C-N bond formation on the aromatic C-H bond, where molecular oxygen is a prerequisite to achieve the catalytic process.
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