期刊
ORGANIC LETTERS
卷 12, 期 6, 页码 1244-1247出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol100113r
关键词
-
资金
- National Institutes of Health [GM-49093]
The tricyclic core of the cylindricine or lepadiformine families of alkaloid natural products was assembled via a Prins addition/intramolecular Schmidt rearrangement under Lewis acid conditions. Both single-pot and two-stage variations of this process were examined, with particular attention to the stereochemical outcome of the processes. This technology has been applied to a formal total synthesis of lepadiformine A and a total synthesis of lepadiformine C.
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