期刊
ORGANIC LETTERS
卷 12, 期 10, 页码 2394-2397出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol100756z
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资金
- F. Hoffman-La Roche Ltd, Basel, Switzerland
A biosynthetically inspired synthesis of (+)-liphagal has been achieved from (+)-sclareolide in 13 steps (9% overall yield). The key step is a biomimetic ring expansion of a highly stabilized benzylic carbocation, which generates the seven-membered ring and the benzofuran of the natural product in a single cascade reaction.
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