期刊
ORGANIC LETTERS
卷 11, 期 7, 页码 1563-1566出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol900171g
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资金
- Ministero dell'Universita e della Ricerca
Allenamides of alpha-amino acids were converted into enantiopure 2-vinylimidazolidin-4-ones by a carbopalladation/exo-cyclization process. The products were obtained in 2.5:1-5.5:1 dr, with 94-99% ee. The palladium-catalyzed carbonylative cyclization of the same substrates afforded enone structures. Starting from properly substituted allenamides, an intramolecular carbopalladation followed by intramolecular amination gave rise to tricyclic fused-ring imidazolidinones.
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