期刊
ORGANIC LETTERS
卷 11, 期 10, 页码 2065-2068出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol900433g
关键词
-
资金
- U.S. Army Research Office [W911NF-07-1-0533]
- Alfred P. Sloan Research Fellow
A counterintuitive observation of a faster signal relay over a longer linear distance prompted detailed kinetic studies of self-immolation reactions. With appropriate conformational bias, trigger-to-reporter signal transduction can take an efficient shortcut that outperforms conventional pathways involving repetitive quinone methide rearrangements and elimination.
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