期刊
ORGANIC LETTERS
卷 11, 期 6, 页码 1197-1200出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol8026768
关键词
-
资金
- NSERC Canada
Masked ortho-benzoquinones are very reactive as diene partners in Diels-Alder reactions. Careful exploration of the orbital factors that govern their surprising behavior shows that their LUMO is almost as electron demanding as that of o-benzoquinone itself, Methyl substituents at either end of their diene system influence the activation energy through modification of the reaction pathway being more or less asynchronous.
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